On the determination of 36Cl and 129I in solid materials from nuclear decommissioning activities

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Authors

Institutes & Expert groups

  • VUB - Vrije Universiteit Brussel
  • DTU - Risoe national laboratory for sustainable energy
  • University of Southampton

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Abstract

Determination of the 36Cl and 129I massic activities using pyrolysis combined with radiochemical separation (using a Clresin) in concrete and graphite samples from decommissioning waste originating from Belgian Reactor 3 and 1 (SCK CEN, Belgium), respectively, is described. Liquid scintillation counting is used for their quantification. The chemical recovery of the procedure was evaluated by determining the stable chlorine with ion chromatography and stable iodine with inductively coupled plasma mass spectrometry. The method was optimized and verified by spiking inactive solid materials.

Details

Original languageEnglish
Pages (from-to)3313–3326
Number of pages14
JournalJournal of Radioanalytical and Nuclear Chemistry
Volume331
DOIs
Publication statusPublished - 21 May 2022

Keywords

  • 36Cl, 129I, Pyrolyser, Cl-resin, LSC, Nuclear decommissioning

ID: 7888942